This photo was recently discovered in the collection. It was taken some time after the Moyne Institute was built (1953) but before the Berkeley Library (1967).
The angle is slightly different, but it may well be related to the 1957 photograph which was used to recruit architects for the design of the Berkeley: https://www.tcd.ie/library/berkeley/5-when-all-this-was-fields/#more-115
Geological Museum - Trinity College Dublin 